210Po and 210Pb radioactivity levels in local and imported tobacco used in Palestine and Jordan.

This study aimed to assess the concentrations of 210Po and 210Pb in various tobacco samples from Palestine and Jordan. Cigarette smoking is recognized as a significant contributor to the radiation dose received by individuals, primarily due to the elevated levels of 210Pb and 210Po found in tobacco. The analysis revealed that the average concentrations of 210Po in locally sourced tobacco and cigarette samples in Palestine are 16.8 ± 2.3 mBq/g and 18.5 ± 2.0 mBq/g, with a total average of 17.8 ± 7.4 mBq/g (15.5 mBq/cigarette). Similarly, the average concentrations of 210Pb in these samples are 18.5 ± 2.6 mBq/g and 20.3 ± 2.2 mBq/g, with a total average of 19.6 ± 8.1 mBq/g (17.0 mBq/cigarette). In Jordan, the average concentrations of 210Po in cigarette samples and narghile tobacco are 20.1 ± 2.4 mBq/g and 18.3 ± 4.1 mBq/g, with a total average value of 19.6 ± 9.9 mBq/g (18.0 mBq/cigarette), while the average concentrations of 210Pb are 22.2 ± 2.6 mBq/g and 20.2 ± 4.5 mBq/g, with a total average value of 21.6 ± 10.8 mBq/g (19.9 mBq/cigarette). The annual effective doses resulting from inhalation were calculated for smokers of these samples. The findings revealed that the levels of 210Po and 210Pb radioactivity in certain investigated samples exceeded the results of studies in many countries of the world. The associated effective doses per year from smoking for all brands products in Palestine range from 34.7 µSv/y to 186.5 µSv/y with an average of 109.5 µSv/y, while in Jordan 54.5 µSv/y to 289.1 µSv/y with an average of 130.9 µSv/y.

Assessment of Be-7, Pb-210 and Po-210 Activities in Airborne Particulate Matter Over Istanbul, Türkiye.

Airborne particulate matter is one of the air pollutants which can have detrimental health effects in the human body. Radionuclides adsorb onto air particles and make their way to humans primarily through inhalation. Naturally-occurring radionuclides, 210Pb and 210Po, are of notable health concern due to their relatively elevated ingestion and inhalation doses. In the current study, activity concentrations of 7Be, 210Pb and 210Po were determined in air particulate matter (PM). PM2.5 was collected on the European side, while PM10 was collected on the Anatolian side of Istanbul. Be-7, 210Pb and 210Po activities were found to be 5.17 ± 2.35, 0.96 ± 0.42; 0.25 ± 0.14 mBq m- 3 in Anatolian side, respectively. Be-7, 210Pb and 210Po activities were found to be 3.81 ± 2.27, 0.62 ± 0.29, 0.29 ± 0.26, mBq m- 3 in European side, respectively. The ratio of 210Po/210Pb was found to be higher (0.47 ± 0.31 for PM2.5 and 0.34 ± 0.27 for PM10) than the global average of 0.1. This result can be explained by the fact that Po is more volatile than Pb and enhanced in the air by the combustion process. Inhalation dose rates of 210Pb and 210Po due to PM10 exposure were calculated to be 7.70 ± 3.30 and 4.05 ± 2.31 µSv year- 1, respectively. Pb-210 bioaccessibility was assessed by the extraction of the particles in simulated lung fluids. Approximately 24.8% of inhaled 210Pb was estimated to be bioaccessible. This study suggests that 210Po and 210Pb activities are partially enhanced in the air particles in Istanbul and should be regularly monitored.

The concentration of radioisotopes (Potassium-40, Polonium-210, Radium-226, and Thorium-230) in fillet tissue carp fishes: A systematic review and probabilistic exposure assessment.

Chemical contamination of seafood has become a global health concern. Carp fish is one of the most widely consumed globally, and several studies have been conducted on the contamination of carp fish with radioisotopes. In the current study, a meta-analysis and probabilistic exposure assessment regarding the Potassium-40 (40K), Polonium-210 (210Po), Radium-226 (226Ra), and Thorium-230 (230Th) in the fillet tissue of carp fish were performed. In this regard, Scopus and PubMed were screened to retrieve the associated citations with on the concentration of radioisotopes in the fillet tissue of carp fish until October 2021. The rank order of radioisotopes in fillet tissue carp fish was 40K (103.49 Bq kg-1) > 210Po (9.39 Bq kg-1) > 226Ra (0.62 Bq kg-1) > 230Th (0.39 Bq kg-1). The highest effective dose due to 210Po ingestion was observed in Spain (male; 4.44E-05 Sv y-1, female; 2.67E-06 Sv y-1); 40K (female, 5.07E-07 Sv y-1); 226Ra (male, 9.93E-09 Sv y-1). The mean of effective dose (ED) in the male and females in India due to ingestion of 230Th as result of carp fish consumption was (1.70E-06 Sv y-1) and (7.01E-08 Sv y-1), respectively. The probabilistic exposure assessment by the Monte Carlo simulation method revealed that consumers of fillet tissue carp fish content of radioisotopes are at a safe range (0.001 Sv y-1).

Review of natural radioactivity in tobacco cigarette brands.

Cigarettes smoking are leading causes of lung cancer in the world. In several countries, the radioactivity of tobaccos cigarette brands has been evaluated to estimate the effective dose from smoking inhalation. In this paper, we have reviewed 40 researched papers of radioactivity in tobacco cigarette brands by searching specified databases from various search engines such as Web of Science, Google Scholar, Scopus, Science Direct and PubMed for the studies published between the year 2000 and November, 2023 in English language. Results show that, the arithmetic mean and range of radioactivity concentration in mBq/g were 20.4 (0.4-128.6), 15.4 (2.0-78.8), 630.8 (1.2-1330.0), 8.1 (0.3-41.0), 15.2 (0.2-82.0) and 5.9 (2.0-16.0) from 210Po, 210Pb, 40K, 232Th and 232U and 226Ra, respectively. The annual effective doses were also estimated using the assumption that a smoker smokes 20 cigarettes per day. The mean annual effective doses in µSv/y from 210Po, 210Pb, 40K, 232Th and 232U and 226Ra were 295, 74.1, 5.80, 889.7, 192.6 and 90.1, respectively. The mean annual effective dose is lower than the reference level 1000 to 20000 µSv/y for existing situation in ICRP Publication 103. The average value of ELCR is 1.03 ×10-3, 0.26 ×10-3,0.02 ×10-3,3.11 ×10-3,0.67 ×10-3 and 0.32 ×10-3 for 210Po, 210Pb, 40K, 232Th and 232U and 226Ra, respectively. The ELCR values obtained in this study are well below the world average value of 1.45 ×10-3. The mean value of LCC in per million is 5.3, 1.3, 0.1, 16, 3.5 and 1.6 for 210Po, 210Pb, 40K, 232Th and 232U and 226Ra, respectively. The values of LCC obtained in this study are all below the limit range of 170-230 per million persons. The result shows 232Th contribute much larger for annual effective dose, annual equivalent dose, ELCR and LCC for smoking tobacco cigarette brands compared to other radionuclides. More studies in radioactivity in tobacco cigarette brands from different countries are required to have conclusive mean annual effective dose, annual equivalent dose, ELCR and LCC for each natural radionuclide.

Distribution of U and 210PO in groundwater of Kodagu district, Karnataka, India.

Trace amounts of uranium along with its decay products are found in varying levels in natural soil, rocks, water and air. They are a matter of significant concern due to their carcinogenic nature. In the present work, the distribution of U and 210Po in groundwater of Kodagu District, Karnataka, India, was studied. The concentration of total U in groundwater samples was estimated using LASER and LED fluorimeter, and the activity of 210Po in groundwater was studied using electrochemical deposition followed by alpha counting method. The concentration of U and 210Po varied from 0.4 to 8.8 µgl-1 and 0.47 to 4.35 mBql-1, respectively. The ingestion dose due to U and 210Po in groundwater varied from 0.33 to 7.17 and 0.41 to 3.81 µSv y-1, respectively. The estimated U activity was found to be well below the standard safe limits of 30 µgl-1 in drinking water, as recommended by WHO and USEPA. The 210Po activity was low compared with the recommended 100 mBql-1 standard of WHO.

Detection of Polonium-210 in Environmental, Biological and Food Samples: A Review.

Ingestion of polonium-210 from environmental media and food can cause serious health hazards (e.g., gastrointestinal symptoms, tumours, etc.) and has been a public health concern worldwide since the 2006 poisoning of Agent Litvinenko 210Po in Russia. With the development of uranium mining and applications of nuclear technology in recent decades, the radioactive hazards posed by 210Po to living organisms and the environment have become increasingly prominent. In order to strengthen the monitoring of environmental 210Po and protect both the environment and human health, a series of explorations on the methods of 210Po determination have been ongoing by researchers across the globe. However, previous reviews have focused on individual sample types and have not provided a comprehensive account of environmental, food, and biological samples that are closely related to human health. In this work, the sources, health hazards, chemical purification, and detection methods of trace 210Po in different sample types are systematically reviewed. In particular, the advantages and disadvantages of various pretreatment methods are compared, and relevant domestic and international standards are integrated, which puts forward a new direction for the subsequent establishment of rapid, simple, and efficient measurement methods.

Factors Contributing to Accumulation of 210Po in Freshwater Fishes in Dong Thai Lake, Vietnam and Radiological Hazard Assessment.

210Po (polonium), one of the most toxic naturally occurring radionuclides, is well-known as a common natural radionuclide in fish species. Human consumption of 210Po-contaminated fish could result in a significant internal dose. This study determined by alpha spectrometry the 210Po activity in sixteen selected fish species with different living behaviors (pelagic, demersal), trophic positions (herbivores, carnivores, omnivorous), and masses in Dong Thai Lake, Hanoi, Vietnam. The min, max, and average of the 210Po concentration of sixteen fish species were 0.80 ± 0.44, 12.7 ± 0.20, and 3.54 ± 0.31 Bq kg-1, respectively. Regarding the different living behaviors, trophic positions, and masses, the results showed trending of 210Popelagic > 210Podemersal; 210Poherbivores < 210Pocarnivores < 210Poomnivorous and 210Po<0.2 kg > 210Po0.2-1 kg > 210Po>1 kg, respectively. The 210Po concentrations in muscle tissue were greater in fish species with a small mass, omnivorous trophic position, and pelagic living behavior relative to demersal fish with a larger mass that were herbivores or carnivores. In addition, the results showed an uneven distribution of 210Po activities in atmospheric aerosols, terrestrial soils, surface waters, and lake sediments in the study area. The primary source of 210Po could be supplied from atmospheric aerosols and/or terrestrial soils in the study area. The 210Po annual effective dose for adults due to fish consumption has been calculated with a range from 20 to 400 µSv y-1 and 111 µSv. y-1 on average, and it is far below the allowable limits of 1000 µSv y-1.

Characteristics of 210Po in Asian overbite clam (Potamocorbula laevis) from the coastal area at Thai Binh province, Vietnam.

210Po concentration in the edible muscle tissue and digestive diverticulum organs of Asian overbite clam at the near-shore Thai Binh, Vietnam was analyzed using alpha detectors. The 210Po activity in muscle tissue and digestive diverticulum organs ranged from 5 ± 1 to 178 ± 10 and from 118 ± 7 to 812 ± 12 Bq.kg-1 with the average value of 25 and 324 Bq.kg-1, respectively. Results showed that 210Po activity in the digestive diverticulum was significantly higher than in the muscle tissue. There was a slightly inverse correlation between 210Po activity in muscle tissue, digestive diverticulum, and clam weight and size. The annual committed effective dose was calculated from 210Po due to the consumption of Asian overbite clam for adults in the study area was higher than the guideline value of 0.2 - 1 mSv.y-1.

Po-210 activity concentrations in wild and farmed fish from the Aegean Sea and Sea of Marmara and dose assessment to consumers.

Polonium (210Po) is the major contributor (with approximately 90%) to the radiation dose from radionuclides contained in the human diet, and it is mostly associated with seafood. This study presents 210Po activity concentrations in the tissues of 16 fish species from the Aegean Sea and Sea of Marmara. Among all species investigated, the highest 210Po activity concentration was 4450 ± 33 Bq kg-1 dry weight (dw) in the digestive tract of anchovy (Engraulis encrasicolus), and the lowest 210Po activity concentration was 1.3 ± 0.6 Bq kg-1 (dw) in the muscle tissue of the thornback ray (Raja clavata). Significant differences in 210Po concentrations were consistently found among the tissues of fish (P < 0.05). In general, the prominent accumulation of 210Po was observed in the digestive tract and liver while the muscle tissue generally displayed the lower concentrations. Polonium concentrations in the internal organs, such as muscle and liver, were related to the feeding ecology of fish and thus are a consequence of 210Po transfer in the food chain rather than 210Po uptake from water. The average 210Po concentration in fish filet was 54.1 Bq kg-1 dw and to attain the recommended limit for the annual committed effective dose (1 mSv year-1) would require the consumption of 1024 kg of mixed fish filet in 1 year, which is unlikely to happen. The highest 210Po activity concentration in the edible part of fish (filet) was determined in the anchovy (E. encrasicolus) but to reach the 1 mSv year-1 limit would require still the consumption of 7.1 kg year-1 of anchovy filet. Similar size specimens of wild and farmed fish, Dicentrarchus labrax and Sparus aurata, were analyzed to assess the differences in 210Po concentrations. Polonium concentrations in the wild fish were several-fold higher than in farmed specimens, these ones fed with fish feed with 210Po content lower than natural food in the sea. Therefore, the current trend of increasing the consumption of seafood from aquaculture seems to be reducing the radiation exposure to 210Po in the human diet that is considered beneficial to public health.

Variation of 210-polonium in the cephalopod community from the Bay of Biscay, North-East Atlantic.

Among natural radionuclides, 210Po is the major contributor to the radiation dose received by marine organisms. In cephalopods, 210Po is concentrated in the digestive gland, which contains over 90% of the whole-body burden of the nuclide. Although previous studies showed that 210Po was taken up independently of 210Pb, its parent nuclide, very little is known about the factors influencing its levels in cephalopods. To the best of our knowledge, no studies investigated 210Po levels in different species at the same time. In the present study, 210Po was analysed in the digestive gland of 62 individuals from 11 species representing a large range of feeding ecologies and habitats, including squids, cuttlefish and octopus species from coastal to deep-oceanic habitats. Among species, the highest activity was measured in Loligo vulgaris (5720 ± 3606 Bq/kg) and the lowest in T. megalops (188 Bq/kg). However, considering the habitats (benthic vs pelagic and neritic vs oceanic), no significant differences appeared. At the species level, no differences between sexes were found so both sexes were plotted together to test the size effect for species with at least 8 individuals (i.e., Eledone cirrhosa, L. vulgaris, L. forbesi and Sepia officinalis). In the first three species, 210Po levels decreased significantly with increasing size or weight but not in S. officinalis. In squid, this could be related to ontogenetic changes in diet from a high proportion of crustaceans (high Po content) in small individuals to fish (low Po content) in larger individuals, while the high dietary plasticity of S. officinalis at all stages of its life cycle could explain the lack of decrease in 210Po with size. In comparison to the few data from the literature, the levels of 210Po concentrations in the cephalopod community of the Bay of Biscay were overall in the same range than those reported in other cephalopods, varying across 4 orders of magnitude. Further studies are needed to understand the mechanism of retention in the cephalopod digestive gland.

Polonium on the 125th anniversary of its discovery: its chemistry, radiotoxicity and application.

The article recounts the discovery of the development of polonium chemistry. The development of its chemistry and the discovery of its properties and uses, both useful and criminal. In addition, it provides biographical details of its discoverers and the scientists who systematically uncovered its secrets.

Seafood dose parameters: Updating 210Po retention factors for cooking, decay loss and mariculture.

210Po has been identified as one of the main contributors to ingestion doses to humans, particularly from the consumption of seafood. The amount of 210Po activity concentration data for various types of seafood has increased greatly in recent times. However, to provide realistic seafood dose assessments, most 210Po data requires correction to account for losses that can occur before the seafood is actually consumed. Here we develop generic correction factors for the main processes associated with reduction of 210Po in seafood - leaching during cooking, radioactive decay between harvest and consumption, and sourcing from mariculture versus wild-caught. When seafood is cooked, the overall mean fraction of 210Po retained is 0.74 for all cooking and seafood types, with the means for various seafood types and cooking categories ranging from 0.56 to 1.03. When considering radioactive decay during the period between harvest and consumption, the overall mean fraction remaining is 0.81 across all seafood preservation/packaging types, with estimates ranging from 0.50 (canned seafood) to 0.98 (fresh seafood). Regarding mariculture influence, the available limited data suggest marine fish and crustaceans raised with processed feed have about one order of magnitude lower (×0.10) 210Po muscle content than wild-caught seafood of the same or similar species, although this ratio varies. Overall, this study concludes that 210Po activity concentrations in seafood at the time of ingestion may be reduced to only about 55% compared to when it was harvested. Therefore, correction factors must be applied to any data derived from environmental monitoring in order to achieve realistic dose estimates. The data also suggest lower 210Po ingestion doses for consumers who routinely favour cooked, long shelf-life and farmed fish/crustaceans. However, more data is needed in some categories, especially for cooking of molluscs and seaweed, and for the 210Po content in all farmed seafood.

Investigation of chemical partitioning of 7Be, 210Pb and 137Cs and novel dating of road sediment by 210Po:210Pb disequilibrium method.

A suite of road sediment and soil samples from a post-industrial city (Detroit, MI) were collected and analyzed for atmospherically-delivered 210Pb, 210Po, 7Be along with 226Ra and 137Cs in the bulk and size-fractionated solid samples. From the measured atmospheric depositional fluxes of 7Be, 210Po, and 210Pb, the initial 210Po/210Pb activity ratio was quantified. In all samples, there is disequilibrium between 210Po and 210Pb, with a 210Po/210Pb activity ratio (AR) of <1.0, which is reported for the first time. Using the measured 210Po/210Pb AR, the average 'apparent age' of road sediment was found to be 146 ± 62 days. Using numerical modeling, it is predicted that the (210Po/210Pb) excess activity ratio will reach a 'dynamic equilibrium' value of ~0.59 over a period of >1 year. Results from a subset of samples that were sequentially extracted for exchangeable, carbonate, Fe-Mn oxide, organic and residual phases indicate the Fe-Mn oxide fraction was found to contain the largest fraction of 7Be and 210Pb; however, the largest fraction of 210Pb was associated with the residual phase and is attributed to complexation of 210Pb with recalcitrant organic matter. This study shows that the natural tagging of 7Be and 210Po-210Pb pair via precipitation provides insights on the time scale of their mobility and adds a new dimension of time information on the pollutant-laden road sediment.

On 210Po and 210Pb in algae diet supplements - The assessed radiation hazard of aquatic superfoods.

Algae are believed to give health benefits. However, the studies showed they contain toxic elements, including radionuclides, and may affect human health. The study presents the values of activity concentrations of 210Po and 210Pb in the algae supplements available worldwide for adults. The activity concentrations (Bq/kg dw) ranged from 0.07 to 14.5 (210Po) and from 0.06 to 8.48 (210Pb). Also, the effective radiation doses and the cancer risk from 210Po and 210Pb decay ingested with analyzed algal supplements have been assessed. The highest values of annual effective doses have been estimated for 210Po in the recommended portion of Spirulina (Arthrospira platensis) from China (59.7 µSv/year) and Diatomaceous earth from the USA (50.4 µSv/year). The cancer morbidity and mortality risk ranged from 10-4 to 10-8. The study indicated the activity concentrations of 210Po and 210Pb were low, and algae supplements for human consumption could be considered safe food.

Study of Polonium (210Po) Activity Concentration in Fruit Wines Derived from Different Locations in Poland.

This study aimed at assessing the activity concentration and the annual effective dose of polonium-210 (210Po) in fruit wines derived from four locations in Poland (Warmian−Masurian, Podlaskie, Lubelskie and Malopolskie voivodeships). The fruit wines differed significantly (p < 0.05) in 210Po activity depending on the production site, with the Malopolskie site having the highest activity (61.4−221.4 mBq/L) and the Podlaskie having the lowest (3.5−97.1 mBq/L). The site differentiation was due to environmental conditions­soil parameters (uranium concentration), precipitations and terrain characteristics, e.g., the proximity of the lakes. The increased activity concentration of 210Po in samples from Malopolska compared with the other sites probably derived from the environment polluted with aqueous wastes and particulate air pollution. The annual effective dose due to the ingestion of fruit wines ranged from 0.112 to 1.214 µSv/year. These levels of exposure are safe according to the WHO criterion (0.1 mSv per year for ingestion) and to the IAEA reference level for public exposure including food (1 mSv per year). Summing up, the data obtained provide information on the activity concentration of 210Po in fruit wines and increase databases on the natural radioactivity of foodstuffs. Future work is needed to examine 210Po activity in samples from all vineyard regions in Poland.

The Concentration of Radionuclides (Lead-210, Polonium-210, and Cesium-137) in the Muscle of Sardine Fish: a Global Systematic Review, Meta-analysis, and Exposure Assessment.

With the increasing use of nuclear technology, concerns about the contamination of water resources with radionuclides and the contamination of seafood are increasing. In the current investigation, a meta-analysis and exposure assessment regarding the concentration of radionuclides, including lead-210 (Pb-210), polonium -210 (Po-210), and cesium-137 (Cs-137) in the muscle of Sardin fish were conducted. In this regard, some databases including Scopus and PubMed were selected to retrieve papers on the concentration of radionuclides in the muscle of Sardin fish from January 2000 to 25 June 2021. The used keywords were polonium-210, natural radioactivity, lead-210, radiocesium, cesium-137, radionuclides, radium-226, seafood, marine foods, fish, sardine fish, sardinella longiceps, and Clupeidae. Also, effective dose (ED) was calculated to estimate carcinogenic risk in Sardine fish consumers. The rank order of radionuclides in the muscle of sardine fish was Po-210 (31.50 Bq/kg) > Pb-210 (3.34 Bq/kg) > Cs-137 (0.48 Bq/kg). Based on level of Pb-210 rank of countries was France (12.00 Bq/kg) > India (4.06 Bq/kg) > Turkey (3.29 Bq/kg) > Spain (1.00 Bq/kg) > Slovenia (0.55 Bq/kg); Po-210 was Turkey (74.96 Bq/kg) > Spain (48.00 Bq/kg) > France (31.500 Bq/kg > India (30.25 Bq/kg) > Slovenia (25.00 Bq/kg) > Kuwait (7.28 Bq/kg) and also, Cs-137 was Japan (1.22 Bq/kg) > Croatia (0.18 Bq/kg) > India (0.23 Bq/kg). The lowest and highest ED of 210Po was observed in Kuwait (5.10E-04 msv/y, female) and France (3.14E-01, male); Pb-210, Slovenia (7.24E-05 msv/y, male) and France (1.48E-02 msv/y, female), and Cs-137, Croatia (8.47E-08 msv/y, male) and Japan (2.54E-05 msv/y, female), respectively. The risk assessment shows that the exposed population are at an acceptable range of risk (H < 1 mSv/y).

Bioaccumulation and retention of Po-210 and Pb-210 in two species of mosses from the zone of influence of the former radium-extracting plants.

The presented study was aimed at assessing the ability to accumulate and retain 210Po and 210Pb in two species of the mosses Sphagnum girgensohnii Russow and Pleurozium schreberi (Willd. ex Brid.) Mitt. Mosses were collected in the zone of influence of the former radium-extracting plants (Komi Republic, Russia). 210Po and 210Pb activity concentrations in S. girgensohnii varied from 131 ± 15.4 to 221 ± 18.3 Bq kg-1, and from 164 ± 18.6 to 309 ± 26.1 Bq kg-1 respectively. In P. schreberi corresponding activity concentrations ranged from 107 ± 18.8 to 328 ± 29.2 Bq kg-1 and from 117 ± 13.2 to 399 ± 31.1 Bq kg-1. Activity concentrations of 210Po and 210Pb in autumn were higher than in summer. In the young parts of the mosses, they were lower than in the old parts. To assess the ability to retain accumulated radionuclides, watersoluble (distilled H2O), exchangeable (1 M CH3COONH4), and acidsoluble (0.1 M H2SO4) fractions of 210Po and 210Pb were isolated from the studied mosses by the method sequential extraction. It was revealed that these fractions in total contained up to 26% of 210Po and 39% of 210Pb. The results showed that the studied moss species are a good biogeochemical barrier and long-term storage for 210Pb and 210Po.

Radiological dose and associated risk due to 210Po in commercial inter-tidal bivalves of southwest (Arabian Sea) coast of India.

The activity concentration of 210Po was determined in edible tissues of commercial bivalves on the southwest coast of India. The 210Po activity ranged from 38.3 ± 6.9 Bq kg-1 to 91.2 ± 18.6 Bq kg-1. The annual committed effective dose (ACED) and lifetime carcinogenic risk (LCR) were calculated for different age groups to determine the potential health risk associated with bivalve consumption. The average ACED ranged from 81.5 to 194.1 µSv y-1, with the 10th and 95th percentiles being 68 and 261 µSv y-1, respectively. Lifelong mortality risk (LMTR) values ranged from 1.2 × 10-3 to 2.9 × 10-3, while lifetime morbidity risk (LMBR) values ranged from 1.9 × 10-6 to 4.9 × 10-6. The effective dose was found to be within the UNSCEAR limits.

Simultaneous determination of 210Pb and 90Sr and 210Po isolation in sludge samples using a plastic scintillation resin.

This study describes a new and fast method for separating 210Po from 210Pb and 90Sr, before simultaneously measuring the individual activities of the latter two radionuclides using a plastic scintillation resin (PSresin) in sludge samples taken from a drinking water treatment plant. This method speeds up the analysis process significantly by simultaneously measuring 210Pb and 90Sr in a single step. The method is reproducible and has a relative standard deviation of less than 25% for 210Pb, 210Po and 90Sr. The method was satisfactorily validated with an intercomparison sample and applied to sludge samples from a drinking water treatment plant. The minimum detectable activities for 0.9 g of sludge are 5.5 Bq/kg and 8 Bq/kg for 210Pb and 90Sr respectively when measured for 180 min, and 0.5 Bq/kg for 210Po when measured for 5000 min.

Determining baseline radiation levels in marine biota - A comparison of SE Queensland commercial species.

Limited data exists on the contribution to radiological dose to members of the public from ingestion of radioactivity in seafood in the Australian diet. There is also a lack of data available to assess the radiological dose to marine fauna in Australian waters. Natural and anthropogenic radionuclides and trace metals were measured in the edible flesh of prawns to determine the radiological dose to humans. The remaining tissues were combined and analysed to enable uptake and environmental radiological doses to be assessed. Although in international studies, the edible flesh is generally measured to determine radiation dose or ingestion of trace metals, the effects of preparation and cooking techniques are rarely assessed. In this study, cooking and preparation techniques that may influence the radiological dose to humans were assessed. Eggs were also removed from a selected number of samples to assess the potential dose in sensitive developmental tissues and possible implications for environmental effects. Order of magnitude differences in 210Po activity concentrations and Cd concentrations were observed between whole animals and the edible flesh of Australian caught King (Melicertus spp.) and Tiger (Penaeus spp.) prawns, with the hepatopancreas primarily responsible for this difference. Most 210Po was unsupported by 210Pb and activity concentrations of all other radionuclides measured (137Cs, 210Pb, 226Ra, 232Th, and 238U) were very low. The major contribution to radiation dose via the ingestion pathway and to the organism itself was from 210Po. Cooking techniques that may lead to leaching of 210Po from the hepatopancreas could substantially increase the radiological dose from ingestion of this isotope. Organism dose estimates using different input assumptions in the radiological assessment tool "ERICA", including site-specific tissue activity concentrations with site- or region-specific media concentrations, were compared with ERICA default distribution coefficients (Kd) and concentration ratios.